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Creators/Authors contains: "Dickerson, Claire E"

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  1. ; ; ; ; ; ; ; ; (, Chemical Science)
    Achieving ultranarrow absorption linewidths in the condensed phase enables optical state preparation of specific non-thermal states, a prerequisite for quantum-enabled technologies. 
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  2. ; ; ; ; ; ; (, The Journal of Physical Chemistry Letters)
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  3. ; ; ; ; ; ; ; ; ; ; et al (, Science)
    The energetic disorder induced by fluctuating liquid environments acts in opposition to the precise control required for coherence-based sensing. Overcoming fluctuations requires a protected quantum subspace that only weakly interacts with the local environment. We report a ytterbium complex that exhibited an ultranarrow absorption linewidth in solution at room temperature with a full width at half maximum of 0.625 milli–electron volts. Using spectral hole burning, we measured an even narrower linewidth of 410 pico–electron volts at 77 kelvin. Narrow linewidths allowed low-field magnetic circular dichroism at room temperature, used to sense Earth-scale magnetic fields. These results demonstrated that ligand protection in lanthanide complexes could substantially diminish electronic state fluctuations. We have termed this system an “atomlike molecular sensor” (ALMS) and proposed approaches to improve its performance. 
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  4. ; ; ; ; ; ; ; ; (, Physical Review Research)
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  5. ; ; ; (, The Journal of Physical Chemistry A)
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  6. ; ; ; ; ; ; ; ; ; ; et al (, ChemRxiv)
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  7. ; ; ; ; ; ; ; ; ; ; et al (, The Journal of Physical Chemistry Letters)
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  8. ; ; ; ; ; ; ; ; ; ; et al (, Nature Chemistry)
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  9. ; ; ; ; (, Journal of the American Chemical Society)
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  10. ; ; ; ; ; ; ; (, The Journal of Physical Chemistry Letters)